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Unit · year 3

PU-306 · Atomic & Molecular Physics

Threads energy · light · matter · waves · fields · symmetry · chance27 lectures18 derivations

Starting from the exact solution of the one-electron atom, the unit builds outward through the hierarchy of corrections — relativistic, spin, nuclear, and external-field — that turn idealized levels into the real spectrum, then confronts electron-electron interaction to explain many-electron atoms and the periodic table. It closes by coupling atoms to the radiation field and to each other, deriving transition rates and selection rules and extending the machinery via Born-Oppenheimer to the rotational, vibrational, and electronic structure of molecules.

PREREQUISITES

PU-104, PU-202, PU-203, PU-204, PU-301

Lectures

L01
The Atomic Scale and the Shape of the Problem
L02
Central Potentials: Separating Radial and Angular Motion
L03
The Hydrogen Atom Solved
L04
Hydrogen Wavefunctions, Degeneracy, and Quantum Numbers
L05
Why Hydrogen Is Not the Whole Story
L06
Relativistic Corrections to the Kinetic Energy
L07
Spin-Orbit Coupling
L08
The Fine Structure of Hydrogen
L09
The Darwin Term and a Glimpse of the Lamb Shift
L10
Hyperfine Structure and the 21 cm Line
L11
Atoms in Magnetic Fields: The Zeeman Effect
L12
Atoms in Electric Fields: The Stark Effect
L13
Identical Particles and Exchange Symmetry
L14
Helium: Ortho, Para, and the Exchange Splitting
L15
Variational Estimates of Atomic Energies
L16
Many-Electron Atoms: The Central-Field Approximation
L17
Hartree-Fock and Self-Consistent Fields
L18
Building the Periodic Table: Term Symbols and Hund's Rules
L19
Radiation and Atoms: Time-Dependent Perturbation Theory
L20
Selection Rules for Dipole Radiation
L21
Einstein Coefficients, Spontaneous Emission, and Lasers
L22
Lineshapes, Widths, and Lifetimes
L23
From Atoms to Molecules: The Born-Oppenheimer Approximation
L24
The Hydrogen Molecular Ion and the Chemical Bond
L25
Molecular Rotation and Vibration
L26
Rovibrational Spectra and the Franck-Condon Principle
L27
Modern Atomic Physics: Laser Cooling and Trapping

Derivations homed in this unit

D-296

Separation of the Central-Potential Schrodinger Equation

Separating a spherically symmetric Hamiltonian into spherical-harmonic angular factors and a one-dimensional radial equation with an effective centrifugal potential.

D-297

Bound-State Spectrum of the Hydrogen Atom

Solving the Coulomb radial equation to obtain E_n = -13.6 eV / n^2, the associated Laguerre wavefunctions, and the n^2 degeneracy.

D-298

Relativistic Kinetic-Energy Correction

Deriving the first-order p^4 correction to hydrogen levels by expanding the relativistic kinetic energy and applying non-degenerate perturbation theory.

D-299

Spin-Orbit Coupling from the Rest Frame

Deriving the L.S interaction from the magnetic field seen in the electron rest frame, including the Thomas precession factor of one half.

D-300

Fine-Structure Energy Formula

Combining the p^4, spin-orbit, and Darwin corrections via degenerate perturbation theory to give levels depending only on n and j.

D-301

Hyperfine Splitting and the 21 cm Line

Deriving the magnetic-dipole coupling between electron and nuclear spins that splits the hydrogen ground state and produces the 21 cm transition.

D-302

Anomalous Zeeman Effect and the Lande g-Factor

Deriving the weak-field Zeeman splitting proportional to the Lande g-factor and its crossover to the Paschen-Back regime.

D-303

Linear Stark Effect in Hydrogen

Using degenerate perturbation theory on the n=2 manifold to obtain a splitting linear in the applied electric field, absent in non-hydrogenic atoms.

D-304

Exchange Symmetry and the Ortho/Para Splitting

Antisymmetrizing the two-electron wavefunction to produce the exchange integral and the singlet-triplet energy splitting of helium.

D-305

Variational Ground-State Energy of Helium

Estimating the helium ground-state energy with a screened-charge trial wavefunction, optimizing the effective nuclear charge.

D-306

The Hartree-Fock Self-Consistent-Field Equations

Deriving the coupled one-electron equations with direct and exchange potentials by minimizing the energy of a Slater determinant.

D-307

LS Coupling, Term Symbols, and Hund's Rules

Ordering many-electron terms by residual electrostatic and spin-orbit energies to justify term symbols and Hund's rules.

D-308

Electric-Dipole Selection Rules

Deriving Delta-l=+/-1 and Delta-m=0,+/-1 and the parity rule from the angular matrix elements of the dipole operator via the Wigner-Eckart theorem.

D-309

Einstein Coefficients and Spontaneous Emission

Relating the A and B coefficients through detailed balance with the Planck spectrum and computing the stimulated rate from Fermi's golden rule.

D-310

The Born-Oppenheimer Approximation

Separating fast electronic from slow nuclear motion using the nuclear-to-electron mass ratio to define potential-energy surfaces.

D-311

The Hydrogen Molecular Ion and the Chemical Bond

Building bonding and antibonding states of H2+ by the LCAO method and showing how electron sharing lowers the energy to bind the nuclei.

D-312

Molecular Rotational and Vibrational Spectra

Deriving rigid-rotor levels B J(J+1) and harmonic plus Morse-anharmonic vibrational levels, and combining them into rovibrational P and R branches.

D-313

The Franck-Condon Principle

Deriving vibronic transition intensities as squared overlaps of vibrational wavefunctions under the assumption of instantaneous electronic transitions.